Quantum Spin-1/2 Rings Built from [2]Triangulene Molecular Units
This study reports the on-surface synthesis and atomic-scale characterization of antiferromagnetic S=1/2 quantum spin rings composed of [2]triangulene units on Au(111), revealing that while planar six-membered rings exhibit uniform excitation gaps describable by a Heisenberg model, distorted five-membered rings display asymmetric spin ground states due to structural distortion-induced degeneracy lifting.
Can Li, Manish Kumar, Ying Wang, Diego Manuel Soler Polo, Yi-Jun Wang, He Qi, Liang Liu, Xiaoxue Liu, Dandan Guan, Yaoyi Li, Hao Zheng, Canhua Liu, Jinfeng Jia, Pei-Nian Liu, Pavel Jelinek, Deng-Yuan (…)2026-02-13🔬 cond-mat.mtrl-sci