Unveiling Davydov-Split Excitons in a Template-Engineered Molecular-Graphene Heterostructure
This study demonstrates that a robust nanofabrication protocol restoring atomic-scale purity to epitaxial graphene on SiC enables the emergence of macroscopic excitonic coherence in HMTP overlayers, revealing a Davydov-split vibronic manifold where a dark excitonic branch dominates radiative relaxation via a polaron-mediated pathway.