Robust Orbital-Selective Flat Bands in Transition-Metal Oxychlorides
This study identifies and experimentally validates a robust, room-temperature orbital-selective flat-band mechanism in van der Waals transition-metal oxychlorides (NbOCl2 and TaOCl2), arising from specific orbital hybridization and Peierls dimerization, thereby establishing a new design principle for realizing exotic quantum phases.