Crystal Anisotropy Implications on the Magneto-Optical Properties of van der Waals FePS3
This study demonstrates that the in-plane structural anisotropy of antiferromagnetic FePS3, driven by distorted FeS6 octahedra, fundamentally governs its magneto-optical properties by dictating the polarization behaviors of distinct electronic transitions from the bulk down to the monolayer limit.
Ellenor Geraffy, Kusha Sharma, Shahar Zuri, Faris Horani, Adam K. Budniak, Muhamed Dawod, Yaron Amouyal, Thomas Brumme, Andrea Maricel León, Thomas Heine, Rajesh Kumar, Doron Naveh, Efrat Lifshitz2026-04-21🔬 cond-mat.mtrl-sci