Tuning the Charge Transfer of Transition Metal Dichalcogenides via Misfit Layer Compounds
This study demonstrates that misfit layer compounds, specifically (LaxPb1-xSe)1.14(NbSe2)2, serve as a versatile platform for precisely tuning electron doping in NbSe2 monolayers through chemical alloying of the rocksalt layer, thereby enabling the engineering of emergent states in 2D transition metal dichalcogenides while preserving their intrinsic electronic structure.