Energies and lifetimes of the 9p and 10p excited states in atomic francium
This paper reports the first experimental measurements of the absolute wavenumbers and radiative lifetimes for the 9p and 10p excited states in francium using Collinear Resonance Ionization Spectroscopy, providing a precise test of relativistic coupled-cluster theory that shows good agreement for lifetimes and relative energies despite a small offset in absolute energies.
P. Lassègues, A. Ajayakumar, M. Athanasakis-Kaklamanakis, O. Ahmad, M. Au, J. Berbalk, D. Bettaney, B. van den Borne, A. Chakraborty, T. E. Cocolios, M. Duggan, C. Fajardo, K. T. Flanagan, R. F. Gar (…)2026-04-15🔬 physics.atom-ph