Tunable Interlayer Charge-Transfer States in MoSe2/WS2 Moiré Superlattices
By combining first-principles calculations and optical spectroscopy, this study demonstrates that a vertical electric field can tune the band alignment of electron-doped MoSe2/WS2 moiré superlattices from Type-I to Type-II, thereby enabling precise control over interlayer charge-transfer states and the realization of a tunable Fermi-Hubbard model with correlated charge-ordered states.